RESUMO
Speciation of tritium (3Ð) in soils from the "Balapan" site in Semipalatinsk are presented in this study. Three interrelated objects were chosen for further study: "Atomic" lake, the Shagan River and an external reservoir. The main speciation forms of 3Ð in soil were: 3Ð in surface-adsorbed water, 3Ð in interlayer water, hydroxylic 3Ð, organically bound 3Ð and crystalline-bound 3Ð. Results will allow an estimation of contamination mechanism to be made, and will also allow the potential for migration and bioavailability of 3Ð to be assessed.
Assuntos
Monitoramento de Radiação/métodos , Poluentes Radioativos do Solo/análise , Trítio/análise , Cazaquistão , Armas Nucleares , SoloRESUMO
This paper provides research data on levels and character of radionuclide contamination distribution in the «sediments- water - plants⯼â¯system of objects of the Semipalatinsk test site (STS). As the research objects there were chosen water bodies of man-made origin which located at the territory of "Experimental Field", "Balapan", "Telkem" and "Sary-Uzen" testing sites. For research the sampling of bottom sediments, water, lakeside and water plants was taken. Collected samples were used to determine concentration of anthropogenic radionuclides 90Sr, 239+240Pu, 241Am, 137Cs. The distribution coefficient (Kd) was calculated as the ratio of the content of radionuclides in the sediments to the content in water, and the concentration ratio (FV) was calculated as the ratio of radionuclide content in plants to the content in sediments or soil.
Assuntos
Monitoramento de Radiação , Poluentes Radioativos da Água/análise , Radioisótopos de Césio/análise , Sedimentos Geológicos , Armas Nucleares , Federação Russa , Radioisótopos de Estrôncio/análiseRESUMO
The Shagan River is the only surface watercourse within the former Semipalatinsk Test Site (STS). Research in the valley of the Shagan River was carried out to study the possible migration of artificial radionuclides with surface waters over considerable distances, with the possibility these radionuclides may have entered the Irtysh River. The investigations revealed that radioactive contamination of soil was primarily caused by the first underground nuclear test with soil outburst conducted at the "Balapan" site in Borehole 1004. The surface nuclear tests carried out at the "Experimental Field" site and global fallout made insignificant contributions to contamination. The most polluted is the area in the immediate vicinity of the "Atomic" Lake crater. Contamination at the site is spatial. The total area of contamination is limited to 10-12 km from the crater piles. The ratio of plutonium isotopes was useful to determine the source of soil contamination. There was virtual absence of artificial radionuclide migration with surface waters, and possible cross-border transfer of radionuclides with the waters of Shagan and Irtysh rivers was not confirmed.